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Opinions?

I dont think the belt squealing was from the alt turning too fast but from a worn belt and or worn pulley(s). If using the old pulleys (if they're good) with a new belt stops the noise you'd be back to normal on the cooling. Yes a bigger/newer rad will help but you need a certain amt of airflow/water flow from a fast enough pulley ratio

live every 24 hour block of time like it's your last day on earth